Raman and Fourier transform infrared spectra of C-H and O-H stretching vibrations in ethanol and its aqueous solutions. Experiment and ab-initio calculations

Jumabaev, A., Absanov, A.A., Hushvaktov, H.A., Xudaykulov, B.B.

O‘zbekiston fizika jurnali · 2024-yil

Annotatsiya

Raman and FTIR spectra of pure ethanol and its proton-donor and proton-acceptor solvents were studied using experiments and ab-initio (DFT) calculations. Spectral bands related to C-H and O-H stretching vibrations of pure ethanol are complex and consist of at least two bands, and these bands belong to different aggregates of ethanol. According to experiments and ab-initio calculations, when ethanol is dissolved in water, the Raman and FTIR spectra related to C-H and O-H stretching vibration shifted towards higher frequency as the concentration of ethanol decreased. This is due to hydrogen bonds in the form of C-H···O (non-classical) and O-H···O. Such shifts take place due to weak interactions between the methyl group in ethanol and water.

Maqola ma’lumotlari
MualliflarJumabaev, A., Absanov, A.A., Hushvaktov, H.A., Xudaykulov, B.B.
JurnalO‘zbekiston fizika jurnali
Nashr sanasi2024-04-08
Jild26
Son1
TilIngliz
DOI10.52304/.v26i1.492

Kalit so‘zlar

комбинационное рассеяние света, FTIR, неэмпирический расчет, этанол, водные растворы, водородные связи, красное смещение, синее смещение, Raman, FTIR spectra, ab-initio calculations, ethanol, aqueous solutions, hydrogen bonding, red-shift, blue-shift

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